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    Strong two-photon absorption at telecommunications wavelengths in nickel bis(dithiolene) complexes

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    cope_285.pdf (138.1Kb)
    Date
    2007-03
    Author
    Cho, Jian-Yang
    Barlow, Stephen
    Marder, Seth R.
    Fu, Jie
    Padilha, Lazaro A.
    Van Stryland, Eric W.
    Hagan, David J.
    Bishop, Maximilienne
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    Abstract
    The two-photon absorption spectrum of a nickel bis(dithiolene) complex with extended conjugation and π-donor substitution is measured by using Z-scan and pump–probe techniques with femtosecond pulses over the spectral range from 1.20to1.58 μm , which includes much of the telecommunications range. The peak two-photon cross section of over 5000 GM (1 GM=10 −50  cm ⁴ sphoton ⁻¹ molecule ⁻¹ ) occurs at ∼1.24 μm , with significant two-photon absorption (>440 GM) throughout the spectral range examined.
    URI
    http://hdl.handle.net/1853/45472
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